Multiscale understanding of high-energy cathodes in solid-state batteries: from atomic scale to macroscopic scale

Shuo Sun; Chenzi Zhao; Hong Yuan; Yang Lu; Jiangkui Hu; Jiaqi Huang; Qiang Zhang

doi:10.1088/2752-5724/ac427c

Topical Review •

OPEN ACCESS

Multiscale understanding of high-energy cathodes in solid-state batteries: from atomic scale to macroscopic scale

doi: 10.1088/2752-5724/ac427c

1 Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, People's Republic of China;
2 Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, People's Republic of China;
3 State Key Laboratory of Automotive Safety and Energy, School of Vehicle and Mobility, Tsinghua University, Beijing 100084, People's Republic of China

基金项目:

This work was supported by National Key Research and Development Program (2021YFB2500300),National Natural Science Foundation of China (22108151, 22075029, 21805161, 21808124, 21825501, 22109084, and U1801257), China Postdoctoral Science Foundation (BX2021135, 2021TQ0164, 2021M701827), Beijing Municipal Natural Science Foundation (Z20J00043), and the ‘Shuimu Tsinghua Scholar Program of Tsinghua University’.

详细信息

通讯作者:

Chen-Zi Zhao, zcz@mail.tsinghua.edu.cn

Qiang Zhang, zhang-qiang@mails.tsinghua.edu.cn

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出版历程
- 收稿日期: 2021-09-30
- 录用日期: 2021-12-13
- 刊出日期: 2022-01-18

Multiscale understanding of high-energy cathodes in solid-state batteries: from atomic scale to macroscopic scale

1 Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, People's Republic of China;
2 Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, People's Republic of China;
3 State Key Laboratory of Automotive Safety and Energy, School of Vehicle and Mobility, Tsinghua University, Beijing 100084, People's Republic of China

Funds:

摘要

摘要:
In the crucial area of sustainable energy storage, solid-state batteries (SSBs) with nonflammable solid electrolytes stand out due to their potential benefits of enhanced safety, energy density, and cycle life. However, the complexity within the composite cathode determines that fabricating an ideal electrode needs to link chemistry (atomic scale), materials (microscopic/mesoscopic scale), and electrode system (macroscopic scale). Therefore, understanding solid-state composite cathodes covering multiple scales is of vital importance for the development of practical SSBs. In this review, the challenges and basic knowledge of composite cathodes from the atomic scale to the macroscopic scale in SSBs are outlined with a special focus on the interfacial structure, charge transport, and mechanical degradation. Based on these dilemmas, emerging strategies to design a high-performance composite cathode and advanced characterization techniques are summarized. Moreover, future perspectives toward composite cathodes are discussed, aiming to facilitate the develop energy-dense SSBs.
- high-energy cathode /
- solid-state battery /
- charge transport /
- advanced characterization /
- solid electrolyte
Abstract:
In the crucial area of sustainable energy storage, solid-state batteries (SSBs) with nonflammable solid electrolytes stand out due to their potential benefits of enhanced safety, energy density, and cycle life. However, the complexity within the composite cathode determines that fabricating an ideal electrode needs to link chemistry (atomic scale), materials (microscopic/mesoscopic scale), and electrode system (macroscopic scale). Therefore, understanding solid-state composite cathodes covering multiple scales is of vital importance for the development of practical SSBs. In this review, the challenges and basic knowledge of composite cathodes from the atomic scale to the macroscopic scale in SSBs are outlined with a special focus on the interfacial structure, charge transport, and mechanical degradation. Based on these dilemmas, emerging strategies to design a high-performance composite cathode and advanced characterization techniques are summarized. Moreover, future perspectives toward composite cathodes are discussed, aiming to facilitate the develop energy-dense SSBs.
- high-energy cathode /
- solid-state battery /
- charge transport /
- advanced characterization /
- solid electrolyte

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参考文献(159)

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Multiscale understanding of high-energy cathodes in solid-state batteries: from atomic scale to macroscopic scale

doi: 10.1088/2752-5724/ac427c

通讯作者:

Chen-Zi Zhao, zcz@mail.tsinghua.edu.cn

Qiang Zhang, zhang-qiang@mails.tsinghua.edu.cn

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Multiscale understanding of high-energy cathodes in solid-state batteries: from atomic scale to macroscopic scale

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Multiscale understanding of high-energy cathodes in solid-state batteries: from atomic scale to macroscopic scale

doi: 10.1088/2752-5724/ac427c

通讯作者: Chen-Zi Zhao, zcz@mail.tsinghua.edu.cn Qiang Zhang, zhang-qiang@mails.tsinghua.edu.cn

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Multiscale understanding of high-energy cathodes in solid-state batteries: from atomic scale to macroscopic scale

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通讯作者:

Chen-Zi Zhao, zcz@mail.tsinghua.edu.cn

Qiang Zhang, zhang-qiang@mails.tsinghua.edu.cn