Volume 3 Issue 1
March  2024
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Jacob Martine, Wissel Kerstin, Clemens Oliver. Recycling of solid-state batterieschallenge and opportunity for a circular economy?[J]. Materials Futures, 2024, 3(1): 012101. doi: 10.1088/2752-5724/acfb28
Citation: Jacob Martine, Wissel Kerstin, Clemens Oliver. Recycling of solid-state batterieschallenge and opportunity for a circular economy?[J]. Materials Futures, 2024, 3(1): 012101. doi: 10.1088/2752-5724/acfb28
Topical Review •
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Recycling of solid-state batterieschallenge and opportunity for a circular economy?

© 2024 The Author(s). Published by IOP Publishing Ltd on behalf of the Songshan Lake Materials Laboratory
Materials Futures, Volume 3, Number 1
  • Received Date: 2023-07-28
  • Accepted Date: 2023-09-18
  • Rev Recd Date: 2023-09-11
  • Publish Date: 2024-01-03
  • The tremendous efforts made in the research field of solid-state Li-ion batteries have led to considerable advancement of this technology and the first market-ready systems can be expected in the near future. The research community is currently investigating different solid-state electrolyte classes (e.g. oxides, sulfides, halides and polymers) with a focus on further optimizing the synthesis and electrochemical performance. However, so far, the development of sustainable recycling strategies allowing for an efficient backflow of critical elements contained in these batteries into the economic cycle and thus a transition from a linear to a circular economy lags behind. In this contribution, resource aspects with respect to the chemical value of crucial materials, which are used for the synthesis of solid-state electrolytes are being discussed. Furthermore, an overview of possible approaches in relation to their challenges and opportunities for the recycling of solid-state batteries with respect to different solid-state electrolyte classes by means of pyrometallurgy, hydrometallurgy and direct recycling/dissolution-based separation processes is given. Based on these considerations and with reference to previous research, it will be shown that different solid-state electrolytes will require individually adapted recycling processes to be suitably designed for a circular economy and that further improvements and investigations will be required.
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  • [1]
    Janek J, Zeier W G 2016 A solid future for battery development Nat. Energy 1 16141 doi: 10.1038/nenergy.2016.141
    [2]
    Lotsch B V, Maier J 2017 Relevance of solid electrolytes for lithium-based batteries: a realistic view J. Electroceramics 38 128-41 doi: 10.1007/s10832-017-0091-0
    [3]
    Kuhn A, Gerbig O, Zhu C, Falkenberg F, Maier J, Lotsch B V 2014 A new ultrafast superionic Li-conductor: ion dynamics in Li11Si2PS12 and comparison with other tetragonal LGPS-type electrolytes Phys. Chem. Chem. Phys. 16 14669-74 doi: 10.1039/C4CP02046D
    [4]
    Thangadurai V, Kaack H, Weppner W J 2003 Novel fast lithium ion conduction in garnet-type Li5La3M2O12 (M= Nb, Ta) J. Am. Ceram. Soc. 86 437-40 doi: 10.1111/j.1151-2916.2003.tb03318.x
    [5]
    Zhu J, et al 2021 End-of-life or second-life options for retired electric vehicle batteries Cell Rep. Phys. Sci. 2 100537 doi: 10.1016/j.xcrp.2021.100537
    [6]
    Shahjalal M, Roy P K, Shams T, Fly A, Chowdhury J I, Ahmed M R, Liu K 2022 A review on second-life of Li-ion batteries: prospects, challenges, and issues Energy 241 122881 doi: 10.1016/j.energy.2021.122881
    [7]
    He Y Q, Yuan X, Zhang G W, Wang H F, Zhang T, Xie W N, Li L P 2021 A critical review of current technologies for the liberation of electrode materials from foils in the recycling process of spent lithium-ion batteries Sci. Total Environ. 766 022025 doi: 10.1016/j.scitotenv.2020.142382
    [8]
    Velzquez-Martnez O, Valio J, Santasalo-Aarnio A, Reuter M, Serna-Guerrero R 2019 A critical review of lithium-ion battery recycling processes from a circular economy perspective Batteries 5 68 doi: 10.3390/batteries5040068
    [9]
    Arshad F, Li L, Amin K, Fan E, Manurkar N, Ahmad A, Yang J, Wu F, Chen R 2020 A comprehensive review of the advancement in recycling the anode and electrolyte from spent lithium ion batteries ACS Sustain. Chem. Eng. 8 13527-54 doi: 10.1021/acssuschemeng.0c04940
    [10]
    Chen Y, Dou A, Zhang Y 2021 A review of recycling status of decommissioned lithium batteries Front. Mater. 8 634667 doi: 10.3389/fmats.2021.634667
    [11]
    Vanderburgt S, Santos R M, Chiang Y W 2023 Is it worthwhile to recover lithium-ion battery electrolyte during lithium-ion battery recycling? Resour. Conserv. Recycl. 189 106733 doi: 10.1016/j.resconrec.2022.106733
    [12]
    Windisch-Kern S, et al 2022 Recycling chains for lithium-ion batteries: a critical examination of current challenges, opportunities and process dependencies Waste Manage. 138 125-39 doi: 10.1016/j.wasman.2021.11.038
    [13]
    Schwich L, Kupers M, Finsterbusch M, Schreiber A, Fattakhova-Rohlfing D, Guillon O, Friedrich B 2020 Recycling strategies for ceramic all-solid-state batteries-part I: study on possible treatments in contrast to Li-ion battery recycling Metals 10 1523 doi: 10.3390/met10111523
    [14]
    Tan D H, Banerjee A, Chen Z, Meng Y S 2020 From nanoscale interface characterization to sustainable energy storage using all-solid-state batteries Nat. Nanotechnol. 15 170-80 doi: 10.1038/s41565-020-0657-x
    [15]
    Tan D H, Xu P, Yang H, M-c K, Nguyen H, Wu E A, Doux J-M, Banerjee A, Meng Y S, Chen Z 2020 Sustainable design of fully recyclable all solid-state batteries MRS Energy Sustain. 7 E23 doi: 10.1557/mre.2020.25
    [16]
    Huang Y X, Qin Z W, Shan C, Xie Y M, Meng X C, Qian D L, He G, Mao D X, Wan L 2023 Green recycling of short-circuited garnet-type electrolyte for high-performance solid-state lithium batteries J. Energy Chem. 80 492-500 doi: 10.1016/j.jechem.2023.01.057
    [17]
    Schneider K, Kiyek V, Finsterbusch M, Yagmurlu B, Goldmann D 2023 Acid leaching of Al-and Ta-substituted Li7La3Zr2O12 (LLZO) solid electrolyte Metals 13 834 doi: 10.3390/met13050834
    [18]
    Chen S J, Hu X C, Nie L, Yu Y, Liu W 2023 Recycling of garnet solid electrolytes with lithium-dendrite penetration by thermal healing Sci. China Mater. 66 2192-8 doi: 10.1007/s40843-022-2371-9
    [19]
    Kononova N, Blmeke S, Cerdas F, Zellmer S, Herrmann C 2023 Identification of target materials for recycling of solid-state batteries from environmental and economic perspective using information theory entropy Proc. CIRP 116 185-90 doi: 10.1016/j.procir.2023.02.032
    [20]
    Abraham M 2015 Prospects and limits of energy storage in batteries J. Phys. Chem. Lett. 6 830-44 doi: 10.1021/jz5026273
    [21]
    Pitek J, Afyon S, Budnyak T M, Budnyk S, Sipponen M H, Slabon A 2021 Sustainable Li-ion batteries: chemistry and recycling Adv. Energy Mater. 11 2003456 doi: 10.1002/aenm.202003456
    [22]
    Chen M Y, Ma X T, Chen B, Arsenault R, Karlson P, Simon N, Wang Y 2019 Recycling end-of-life electric vehicle lithium-ion batteries Joule 3 2622-46 doi: 10.1016/j.joule.2019.09.014
    [23]
    Bai Y C, Muralidharan N, Sun Y-K, Passerini S, Whittingham M S, Belharouak I 2020 Energy and environmental aspects in recycling lithium-ion batteries: concept of battery identity global passport Mater. Today 41 304-15 doi: 10.1016/j.mattod.2020.09.001
    [24]
    Yang J, Fan E, Lin J, Arshad F, Zhang X, Wang H, Wu F, Chen R, Li L 2021 Recovery and reuse of anode graphite from spent lithium-ion batteries via citric acid leaching ACS Appl. Energy Mater. 4 6261-8 doi: 10.1021/acsaem.1c01029
    [25]
    Neumann J, Petranikova M, Meeus M, Gamarra J D, Younesi R, Winter M, Nowak S 2022 Recycling of lithium-ion batteries-current state of the art, circular economy, and next generation recycling Adv. Energy Mater. 12 2102917 doi: 10.1002/aenm.202102917
    [26]
    Yu D, Huang Z, Makuza B, Guo X, Tian Q 2021 Pretreatment options for the recycling of spent lithium-ion batteries: a comprehensive review Miner. Eng. 173 107218 doi: 10.1016/j.mineng.2021.107218
    [27]
    Zhang X, Li L, Fan E, Xue Q, Bian Y, Wu F, Chen R 2018 Toward sustainable and systematic recycling of spent rechargeable batteries Chem. Soc. Rev. 47 7239-302 doi: 10.1039/c8cs00297e
    [28]
    Dunn J B, Gaines L, Sullivan J, Wang M Q 2012 Impact of recycling on cradle-to-gate energy consumption and greenhouse gas emissions of automotive lithium-ion batteries Environ. Sci. Technol. 46 12704-10 doi: 10.1021/es302420z
    [29]
    Li J, Wang G, Xu Z 2016 Environmentally-friendly oxygen-free roasting/wet magnetic separation technology for in situ recycling cobalt, lithium carbonate and graphite from spent LiCoO2/graphite lithium batteries J. Hazard. Mater. 302 97-104 doi: 10.1016/j.jhazmat.2015.09.050
    [30]
    Xiao J, Li J, Xu Z 2017 Recycling metals from lithium ion battery by mechanical separation and vacuum metallurgy J. Hazard. Mater. 338 124-31 doi: 10.1016/j.jhazmat.2017.05.024
    [31]
    Wang D H, Wen H, Chen H J, Yang Y J, Liang H Y 2016 Chemical evolution of LiCoO2 and NaHSO4 center dot H2O mixtures with different mixing ratios during roasting process Chem. Res. Chin. Univ. 32 674-7 doi: 10.1007/s40242-016-5490-2
    [32]
    Fan E, Li L, Wang Z, Lin J, Huang Y, Yao Y, Chen R, Wu F 2020 Sustainable recycling technology for Li-ion batteries and beyond: challenges and future prospects Chem. Rev. 120 7020-63 doi: 10.1021/acs.chemrev.9b00535
    [33]
    Barik S P, Prabaharan G, Kumar L 2017 Leaching and separation of Co and Mn from electrode materials of spent lithium-ion batteries using hydrochloric acid: laboratory and pilot scale study J. Clean. Prod. 147 37-43 doi: 10.1016/j.jclepro.2017.01.095
    [34]
    Wang R-C, Lin Y-C, Wu S-H 2009 A novel recovery process of metal values from the cathode active materials of the lithium-ion secondary batteries Hydrometallurgy 99 194-201 doi: 10.1016/j.hydromet.2009.08.005
    [35]
    Zhang P W, Yokoyama T, Itabashi O, Suzuki T M, Inoue K 1998 Hydrometallurgical process for recovery of metal values from spent lithium-ion secondary batteries Hydrometallurgy 47 259-71 doi: 10.1016/S0304-386X(97)00050-9
    [36]
    Tang W J, Chen X P, Zhou T, Duan H, Chen Y B, Wang J 2014 Recovery of Ti and Li from spent lithium titanate cathodes by a hydrometallurgical process Hydrometallurgy 147 210-6 doi: 10.1016/j.hydromet.2014.05.013
    [37]
    Nan J M, Han D M, Zuo X X 2005 Recovery of metal values from spent lithium-ion batteries with chemical deposition and solvent extraction J. Power Sources 152 278-84 doi: 10.1016/j.jpowsour.2005.03.134
    [38]
    Fan X P, Song C H, Lu X F, Shi Y, Yang S L, Zheng F H, Huang Y G, Liu K, Wang H Q, Li Q Y 2021 Separation and recovery of valuable metals from spent lithium-ion batteries via concentrated sulfuric acid leaching and regeneration of LiNi1/3Co1/3Mn1/3O2 J. Alloys Compd. 863 158775 doi: 10.1016/j.jallcom.2021.158775
    [39]
    Meshram P, Pandey B D, Mankhand T R 2015 Hydrometallurgical processing of spent lithium ion batteries (LIBs) in the presence of a reducing agent with emphasis on kinetics of leaching Chem. Eng. J. 281 418-27 doi: 10.1016/j.cej.2015.06.071
    [40]
    Li H, Xing S Z, Liu Y, Li F J, Guo H, Kuang G 2017 Recovery of lithium, iron, and phosphorus from spent LiFePO4 batteries using stoichiometric sulfuric acid leaching system ACS Sustain. Chem. Eng. 5 8017-24 doi: 10.1021/acssuschemeng.7b01594
    [41]
    Lee C K, Rhee K-I 2002 Preparation of LiCoO2 from spent lithium-ion batteries J. Power Sources 109 17-21 doi: 10.1016/S0378-7753(02)00037-X
    [42]
    Lee C K, Rhee K-I 2003 Reductive leaching of cathodic active materials from lithium ion battery wastes Hydrometallurgy 68 5-10 doi: 10.1016/S0304-386X(02)00167-6
    [43]
    Pinna E G, Ruiz M C, Ojeda M W, Rodriguez M H 2017 Cathodes of spent Li-ion batteries: dissolution with phosphoric acid and recovery of lithium and cobalt from leach liquors Hydrometallurgy 167 66-71 doi: 10.1016/j.hydromet.2016.10.024
    [44]
    Chen X, Ma H, Luo C, Zhou T 2017 Recovery of valuable metals from waste cathode materials of spent lithium-ion batteries using mild phosphoric acid J. Hazard. Mater. 326 77-86 doi: 10.1016/j.jhazmat.2016.12.021
    [45]
    Dong X Y, Huang X R, Tang R, Min Y L, Xu Q J, Hu Z H, Shi P H 2023 Efficient photo-oxidation leaching of Ni and Co in a spent lithium-ion battery cathode by homogeneous UV/H2O2 ACS Sustain. Chem. Eng. 11 9330-6 doi: 10.1021/acssuschemeng.3c00390
    [46]
    Qi Y P, Meng F S, Yi X X, Shu J C, Chen M J, Sun Z, Sun S H, Xiu F-R 2020 A novel and efficient ammonia leaching method for recycling waste lithium ion batteries J. Clean. Prod. 251 119665 doi: 10.1016/j.jclepro.2019.119665
    [47]
    Li D M, Zhang B, Ou X, Zhang J F, Meng K, Ji G J, Li P F, Xu J H 2021 Ammonia leaching mechanism and kinetics of LiCoO2 material from spent lithium-ion batteries Chin. Chem. Lett. 32 2333-7 doi: 10.1016/j.cclet.2020.11.074
    [48]
    Ku H, Jung Y, Jo M, Park S, Kim S, Yang D, Rhee K, An E-M, Sohn J, Kwon K 2016 Recycling of spent lithium-ion battery cathode materials by ammoniacal leaching J. Hazard. Mater. 313 138-46 doi: 10.1016/j.jhazmat.2016.03.062
    [49]
    Almeida J R, Moura M N, Barrada R V, Barbieri E M S, Carneiro M, Ferreira S A D, Lelis M F F, de Freitas M, Brandao G P 2019 Composition analysis of the cathode active material of spent Li-ion batteries leached in citric acid solution: a study to monitor and assist recycling processes Sci. Total Environ. 685 589-95 doi: 10.1016/j.scitotenv.2019.05.243
    [50]
    Yu M, Zhang Z H, Xue F, Yang B, Guo G H, Qiu J H 2019 A more simple and efficient process for recovery of cobalt and lithium from spent lithium-ion batteries with citric acid Sep. Purif. Technol. 215 398-402 doi: 10.1016/j.seppur.2019.01.027
    [51]
    Li L, Ge J, Wu F, Chen R J, Chen S, Wu B R 2010 Recovery of cobalt and lithium from spent lithium ion batteries using organic citric acid as leachant J. Hazard. Mater. 176 288-93 doi: 10.1016/j.jhazmat.2009.11.026
    [52]
    Setiawan H, Petrus H T B M, Perdana I 2019 Reaction kinetics modeling for lithium and cobalt recovery from spent lithium-ion batteries using acetic acid Int. J. Miner. Metall. Mater. 26 98-107 doi: 10.1007/s12613-019-1713-0
    [53]
    Zhang Z M, He W Z, Li G M, Xia J, Hu H K, Huang J W 2014 Ultrasound-assisted hydrothermal renovation of LiCoO2 from the cathode of spent lithium-ion batteries Int. J. Electrochem. Sci. 9 3691-700 doi: 10.1016/S1452-3981(23)08042-2
    [54]
    Ganter M J, Landi B J, Babbitt C W, Anctil A, Gaustad G 2014 Cathode refunctionalization as a lithium ion battery recycling alternative J. Power Sources 256 274-80 doi: 10.1016/j.jpowsour.2014.01.078
    [55]
    Ciez R E, Whitacre J F 2019 Examining different recycling processes for lithium-ion batteries Nat. Sustain. 2 148-56 doi: 10.1038/s41893-019-0222-5
    [56]
    Zhang Z Z, et al 2018 New horizons for inorganic solid state ion conductors Energy Environ. Sci. 11 1945-76 doi: 10.1039/C8EE01053F
    [57]
    Zhou D, Shanmukaraj D, Tkacheva A, Armand M, Wang G 2019 Polymer electrolytes for lithium-based batteries: advances and prospects Chemistry 5 2326-52 doi: 10.1016/j.chempr.2019.05.009
    [58]
    Gao Z, Sun H, Fu L, Ye F, Zhang Y, Luo W, Huang Y 2018 Promises, challenges, and recent progress of inorganic solid-state electrolytes for all-solid-state lithium batteries Adv. Mater. 30 e1705702 doi: 10.1002/adma.201705702
    [59]
    Zeier W G 2014 Structural limitations for optimizing garnet-type solid electrolytes: a perspective Dalton Trans. 43 16133-8 doi: 10.1039/C4DT02162B
    [60]
    Bates J, Dudney N J, Gruzalski G R, Zuhr R A, Choudhury A, Luck C F, Robertson J D 1992 Electrical properties of amorphous lithium electrolyte thin films Solid State Ionics 53-56 647-54 doi: 10.1016/0167-2738(92)90442-R
    [61]
    Kwon W J, Kim H, Jung K-N, Cho W, Kim S H, Lee J-W, Park M-S 2017 Enhanced Li+ conduction in perovskite Li3xLa2/3x1/32xTiO3 solid-electrolytes via microstructural engineering J. Mater. Chem. A 5 6257-62 doi: 10.1039/C7TA00196G
    [62]
    DeWees R, Wang H 2019 Synthesis and properties of NaSICON-type LATP and LAGP solid electrolytes ChemSusChem 12 3713-25 doi: 10.1002/cssc.201900725
    [63]
    Howard M A, Clemens O, Knight K S, Anderson P A, Hafiz S, Panchmatia P M, Slater P R 2013 Synthesis, conductivity and structural aspects of Nd3Zr2Li7-3xAlxO12 J. Mater. Chem. A 1 14013-22 doi: 10.1039/c3ta13252h
    [64]
    Waetzig K, Rost A, Heubner C, Coeler M, Nikolowski K, Wolter M, Schilm J 2020 Synthesis and sintering of Li1.3Al0.3Ti1.7(PO43 (LATP) electrolyte for ceramics with improved Li+ conductivity J. Alloys Compd. 818 153237 doi: 10.1016/j.jallcom.2019.153237
    [65]
    Djenadic R, Botros M, Benel C, Clemens O, Indris S, Choudhary A, Bergfeldt T, Hahn H 2014 Nebulized spray pyrolysis of Al-doped Li7La3Zr2O12 solid electrolyte for battery applications Solid State Ionics 263 49-56 doi: 10.1016/j.ssi.2014.05.007
    [66]
    Botros M, Djenadic R, Clemens O, Mller M, Hahn H 2016 Field assisted sintering of fine-grained Li7-3xLa3Zr2AlxO12 solid electrolyte and the influence of the microstructure on the electrochemical performance J. Power Sources 309 108-15 doi: 10.1016/j.jpowsour.2016.01.086
    [67]
    Lobe S, Bauer A, Sebold D, Wettengl N, Fattakhova-Rohlfing D, Uhlenbruck S 2022 Sintering of Li-garnets: impact of Al-incorporation and powder-bed composition on microstructure and ionic conductivity Open Ceram. 10 100268 doi: 10.1016/j.oceram.2022.100268
    [68]
    Koerver R, Zhang W, de Biasi L, Schweidler S, Kondrakov A O, Kolling S, Brezesinski T, Hartmann P, Zeier W G, Janek J 2018 Chemo-mechanical expansion of lithium electrode materialson the route to mechanically optimized all-solid-state batteries Energy Environ. Sci. 11 2142-58 doi: 10.1039/C8EE00907D
    [69]
    Koerver R, Aygn I, Leichtwei T, Dietrich C, Zhang W, Binder J O, Hartmann P, Zeier W G, Janek J 2017 Capacity fade in solid-state batteries: interphase formation and chemomechanical processes in nickel-rich layered oxide cathodes and lithium thiophosphate solid electrolytes Chem. Mater. 29 5574-82 doi: 10.1021/acs.chemmater.7b00931
    [70]
    Chen L, Li Y, Li S-P, Fan L-Z, Nan C-W, Goodenough J B 2018 PEO/garnet composite electrolytes for solid-state lithium batteries: from ceramic-in-polymer to polymer-in-ceramic Nano Energy 46 176-84 doi: 10.1016/j.nanoen.2017.12.037
    [71]
    Fingerle M, Loho C, Ferber T, Hahn H, Hausbrand R 2017 Evidence of the chemical stability of the garnet-type solid electrolyte Li5La3Ta2O12 towards lithium by a surface science approach J. Power Sources 366 72-79 doi: 10.1016/j.jpowsour.2017.08.109
    [72]
    Liu Z, Fu W, Payzant E A, Yu X, Wu Z, Dudney N J, Kiggans J, Hong K, Rondinone A J, Liang C 2013 Anomalous high ionic conductivity of nanoporous beta-Li3PS4 J. Am. Chem. Soc. 135 975-8 doi: 10.1021/ja3110895
    [73]
    Deiseroth H-J, Kong S-T, Eckert H, Vannahme J, Reiner C, Zaiss T, Schlosser M 2008 Li6PS5X: a class of crystalline Li-rich solids with an unusually high Li+ mobility Angew. Chem., Int. Ed. 47 755-8 doi: 10.1002/anie.200703900
    [74]
    Kamaya N, et al 2011 A lithium superionic conductor Nat. Mater. 10 682-6 doi: 10.1038/nmat3066
    [75]
    Wingender J, Redaktion R, Hartwig A 2013 Phosphor RÖMPP. Thieme Gruppe(available at: https://roempp.thieme.de/lexicon/RD-16-01961)(Accessed 16 October 2023)
    [76]
    Yamamoto K, et al 2021 High ionic conductivity of liquid-phase-synthesized Li3PS4 solid electrolyte, comparable to that obtained via ball milling ACS Appl. Energy Mater. 4 2275-81 doi: 10.1021/acsaem.0c02771
    [77]
    Li X, Liang J, Yang X, Adair K R, Wang C, Zhao F, Sun X 2020 Progress and perspectives on halide lithium conductors for all-solid-state lithium batteries Energy Environ. Sci. 13 1429-61 doi: 10.1039/C9EE03828K
    [78]
    Braga M H, Ferreira J A, Stockhausen V, Oliveira J E, El-Azab A 2014 Novel Li3ClO based glasses with superionic properties for lithium batteries J. Mater. Chem. A 2 5470-80 doi: 10.1039/C3TA15087A
    [79]
    Kwak H, et al 2021 New cost-effective halide solid electrolytes for all-solid-state batteries: mechanochemically prepared Fe3+-substituted Li2ZrCl6 Adv. Energy Mater. 11 2003190 doi: 10.1002/aenm.202003190
    [80]
    Li X, et al 2019 Air-stable Li3InCl6 electrolyte with high voltage compatibility for all-solid-state batteries Energy Environ. Sci. 12 2665-71 doi: 10.1039/C9EE02311A
    [81]
    Heenen H H, Voss J, Scheurer C, Reuter K, Luntz A C 2019 Multi-ion conduction in Li3OCl glass electrolytes J. Phys. Chem. Lett. 10 2264-9 doi: 10.1021/acs.jpclett.9b00500
    [82]
    Zhao Y, Daemen L L 2012 Superionic conductivity in lithium-rich anti-perovskites J. Am. Chem. Soc. 134 15042-7 doi: 10.1021/ja305709z
    [83]
    Li X, et al 2019 Water-mediated synthesis of a superionic halide solid electrolyte Angew. Chem. 131 16579-84 doi: 10.1002/ange.201909805
    [84]
    Wang C, et al 2021 A universal wet-chemistry synthesis of solid-state halide electrolytes for all-solid-state lithium-metal batteries Sci. Adv. 7 eabh1896 doi: 10.1126/sciadv.abh1896
    [85]
    Arya A, Sharma A L 2020 A glimpse on all-solid-state Li-ion battery (ASSLIB) performance based on novel solid polymer electrolytes: a topical review J. Mater. Sci. 55 6242-304 doi: 10.1007/s10853-020-04434-8
    [86]
    Zhao Y, Wang L, Zhou Y, Liang Z, Tavajohi N, Li B, Li T 2021 Solid polymer electrolytes with high conductivity and transference number of Li ions for Li-based rechargeable batteries Adv. Sci. 8 2003675 doi: 10.1002/advs.202003675
    [87]
    Sashmitha K, Rani M U 2023 A comprehensive review of polymer electrolyte for lithium-ion battery Polym. Bull. 80 89-135 doi: 10.1007/s00289-021-04008-x
    [88]
    Ravve A 2012 Principles of Polymer ChemistrySpringer doi: 10.1002/pola.25955
    [89]
    Peacock A J, Calhoun A 2012 Polymer Chemistry: Properties and ApplicationCarl Hanser Verlag GmbH & Company KG
    [90]
    Ye F, Liao K, Ran R, Shao Z 2020 Recent advances in filler engineering of polymer electrolytes for solid-state Li-ion batteries: a review Energy Fuels 34 9189-207 doi: 10.1021/acs.energyfuels.0c02111
    [91]
    Waidha A I, Ferber T, Donzelli M, Hosseinpourkahvaz N, Vanita V, Dirnberger K, Ludwigs S, Hausbrand R, Jaegermann W, Clemens O 2021 Compositional dependence of Li-ion conductivity in garnet-rich composite electrolytes for all-solid-state lithium-ion batteries-toward understanding the drawbacks of ceramic-rich composites ACS Appl. Mater. Interfaces 13 31111-28 doi: 10.1021/acsami.1c05846
    [92]
    Hees T, Zhong F, Sturzel M, Mulhaupt R 2019 Tailoring hydrocarbon polymers and all-hydrocarbon composites for circular economy Macromol. Rapid Commun. 40 e1800608 doi: 10.1002/marc.201800608
    [93]
    Doose S, Mayer J K, Michalowski P, Kwade A 2021 Challenges in ecofriendly battery recycling and closed material cycles: a perspective on future lithium battery generations Metals 11 291 doi: 10.3390/met11020291
    [94]
    Miara L, Windmuller A, Tsai C-L, Richards W D, Ma Q, Uhlenbruck S, Guillon O, Ceder G 2016 About the compatibility between high voltage spinel cathode materials and solid oxide electrolytes as a function of temperature ACS Appl. Mater. Interfaces 8 26842-50 doi: 10.1021/acsami.6b09059
    [95]
    Gellert M, Dashjav E, Grner D, Ma Q, Tietz F 2017 Compatibility study of oxide and olivine cathode materials with lithium aluminum titanium phosphate Ionics 24 1001-6 doi: 10.1007/s11581-017-2276-6
    [96]
    Rumpel M, Nagler F, Appold L, Stracke W, Flegler A, Clemens O, Sextl G 2022 Thermal stabilities of Mn-based active materials in combination with the ceramic electrolyte LATP for ASSB bulk cathodes Mater. Adv. 3 4015-25 doi: 10.1039/D2MA00158F
    [97]
    Wiberg N 2008 Lehrbuch der Anorganischen Chemie102 ednDe Gruyter doi: 10.1515/9783110177701
    [98]
    Redaktion R 2002 Zirconium RÖMPP. Thieme Gruppe(available at: https://roempp.thieme.de/lexicon/RD-26-00467)(Accessed 16 October 2023)
    [99]
    Schirmer T, Qiu H, Goldmann D, Stallmeister C, Friedrich B 2022 Influence of P and Ti on phase formation at solidification of synthetic slag containing Li, Zr, La, and Ta Minerals 12 310 doi: 10.3390/min12030310
    [100]
    Geeson M B, Cummins C C 2020 Let’s make white phosphorus obsolete ACS Central Sci. 6 848-60 doi: 10.1021/acscentsci.0c00332
    [101]
    Heitmann A, Reher P 1974 Recycling-Prozesse fr Schwefel-Verbindungen Chem. Ing. Tech. 46 589-94 doi: 10.1002/cite.330461403
    [102]
    Blengini G A, et alEuropean Commission 2020 Study on the EU’s list of critical raw materialsfinal report (Publications Office of the European Union)10.2873/11619
    [103]
    Oelkers B 2002 Zirconiumchloride RÖMPP. Thieme Gruppe(available at: https://roempp.thieme.de/lexicon/RD-26-00469)(Accessed 16 October 2023)
    [104]
    Redaktion R 2002 Yttrium-Verbindungen RÖMPP. Thieme Gruppe(available at: https://roempp.thieme.de/lexicon/RD-25-00067)(Accessed 16 October 2023)
    [105]
    Vohldal J 2021 Polymer degradation: a short review Chem. Teach. Int. 3 213-20 doi: 10.1515/cti-2020-0015
    [106]
    Nisar A, Khan S, Hameed M, Nisar A, Ahmad H, Mehmood S A 2021 Bio-conversion of CO2 into biofuels and other value-added chemicals via metabolic engineering Microbiol. Res. 251 126813 doi: 10.1016/j.micres.2021.126813
    [107]
    Saleh H M, Hassan A I 2023 Green conversion of carbon dioxide and sustainable fuel synthesis Fire 6 128 doi: 10.3390/fire6030128
    [108]
    Ali Nowroozi M, Iqbal Waidha A, Jacob M, van Aken P A, Predel F, Ensinger W, Clemens O 2022 Towards recycling of LLZO solid electrolyte exemplarily performed on LFP/LLZO/LTO cells ChemistryOpen 11 e202100274 doi: 10.1002/open.202100274
    [109]
    Falcn H, Goeta A E, Punte G, Carbonio R E 1997 Crystal structure refinement and stability of LaFexNi1-xO3 solid solutions J. Solid State Chem. 133 379-85 doi: 10.1006/jssc.1997.7477
    [110]
    Rodrguez-Carvajal J, Hennion M, Moussa F, Moudden A H, Pinsard L, Revcolevschi A 1998 Neutron-diffraction study of the Jahn-Teller transition in stoichiometric LaMnO3 Phys. Rev. B 57 R3189-92 doi: 10.1103/PhysRevB.57.R3189
    [111]
    Thornton G, Tofield B C, Hewat A W 1986 A neutron diffraction study of LaCoO3 in the temperature range 4.2 < T < 1248 K J. Solid State Chem. 61 301-7 doi: 10.1016/0022-4596(86)90035-6
    [112]
    Bhatia H, Thieu D T, Pohl A H, Chakravadhanula V S K, Fawey M H, Kubel C, Fichtner M 2017 Conductivity optimization of tysonite-type La1-xBaxF3-x solid electrolytes for advanced fluoride ion battery ACS Appl. Mater. Interfaces 9 23707-15 doi: 10.1021/acsami.7b04936
    [113]
    Holleman A F, Wiberg N 1995 Lehrbuch der Anorganischen Chemie101 edndeGruyter doi: 10.1002/ange.19961082135
    [114]
    Bae H, Kim Y 2021 Technologies of lithium recycling from waste lithium ion batteries: a review Mater. Adv. 2 3234-50 doi: 10.1039/D1MA00216C
    [115]
    Waidha A I, et al 2023 Recycling of all-solid-state li-ion batteries: a case study of the separation of individual components within a system composed of LTO, LLZTO and NMC ChemSusChem 16 e202202361 doi: 10.1002/cssc.202202361
    [116]
    Ghidiu M, Ruhl J, Culver S P, Zeier W G 2019 Solution-based synthesis of lithium thiophosphate superionic conductors for solid-state batteries: a chemistry perspective J. Mater. Chem. A 7 17735-53 doi: 10.1039/C9TA04772G
    [117]
    Nikodimos Y, Huang C-J, Taklu B W, Su W-N, Hwang B J 2022 Chemical stability of sulfide solid-state electrolytes: stability toward humid air and compatibility with solvents and binders Energy Environ. Sci. 15 991-1033 doi: 10.1039/D1EE03032A
    [118]
    Prayog L D, Faisal M, Kartini E, Hoggowiranto W, Supardi S 2016 Morphology and conductivity study of solid electrolyte Li3PO4 AIP Conf. Proc. 1710 030047 doi: 10.1063/1.4941513
    [119]
    Stffler H, et al 2019 Amorphous versus crystalline Li3PS4: local structural changes during synthesis and Li ion mobility J. Phys. Chem. C 123 10280-90 doi: 10.1021/acs.jpcc.9b01425
    [120]
    Dietrich C, Weber D A, Culver S, Senyshyn A, Sedlmaier S J, Indris S, Janek J, Zeier W G 2017 Synthesis, structural characterization, and lithium ion conductivity of the lithium thiophosphate Li2P2S6 Inorg. Chem. 56 6681-7 doi: 10.1021/acs.inorgchem.7b00751
    [121]
    Dietrich C, Weber D A, Sedlmaier S J, Indris S, Culver S P, Walter D, Janek J, Zeier W G 2017 Lithium ion conductivity in Li2S-P2S5 glassesbuilding units and local structure evolution during the crystallization of superionic conductors Li3PS4, Li7P3S11 and Li4P2S7 J. Mater. Chem. A 5 18111-9 doi: 10.1039/C7TA06067J
    [122]
    Kuhn A, Duppel V, Lotsch B V 2013 Tetragonal Li10GeP2S12 and Li7GePS8exploring the Li ion dynamics in LGPS Li electrolytes Energy Environ. Sci. 6 3548-52 doi: 10.1039/c3ee41728j
    [123]
    Calpa M, Nakajima H, Mori S, Goto Y, Mizuguchi Y, Moriyoshi C, Kuroiwa Y, Rosero-Navarro N C, Miura A, Tadanaga K 2021 Formation mechanism of -Li3PS4 through decomposition of complexes Inorg. Chem. 60 6964-70 doi: 10.1021/acs.inorgchem.1c00294
    [124]
    Wang H, Hood Z D, Xia Y, Liang C 2016 Fabrication of ultrathin solid electrolyte membranes of -Li3PS4 nanoflakes by evaporation-induced self-assembly for all-solid-state batteries J. Mater. Chem. A 4 8091-6 doi: 10.1039/C6TA02294D
    [125]
    Hikima K, Ogawa K, Gamo H, Matsuda A 2023 Li10GeP2S12 solid electrolytes synthesised via liquid-phase methods Chem. Commun. 59 6564-7 doi: 10.1039/D3CC01018J
    [126]
    Yubuchi S, Teragawa S, Aso K, Tadanaga K, Hayashi A, Tatsumisago M 2015 Preparation of high lithium-ion conducting Li6PS5Cl solid electrolyte from ethanol solution for all-solid-state lithium batteries J. Power Sources 293 941-5 doi: 10.1016/j.jpowsour.2015.05.093
    [127]
    Yubuchi S, Uematsu M, Hotehama C, Sakuda A, Hayashi A, Tatsumisago M 2019 An argyrodite sulfide-based superionic conductor synthesized by a liquid-phase technique with tetrahydrofuran and ethanol J. Mater. Chem. A 7 558-66 doi: 10.1039/C8TA09477B
    [128]
    Teragawa S, Aso K, Tadanaga K, Hayashi A, Tatsumisago M 2013 Formation of Li2S-P2S5 solid electrolyte from N-methylformamide solution Chem. Lett. 42 1435-7 doi: 10.1246/cl.130726
    [129]
    Teragawa S, Aso K, Tadanaga K, Hayashi A, Tatsumisago M 2014 Preparation of Li2S-P2S5 solid electrolyte from N-methylformamide solution and application for all-solid-state lithium battery J. Power Sources 248 939-42 doi: 10.1016/j.jpowsour.2013.09.117
    [130]
    Zhou L, Park K-H, Sun X, Lalre F, Adermann T, Hartmann P, Nazar L F 2018 Solvent-engineered design of argyrodite Li6PS5X (X = Cl, Br, I) solid electrolytes with high ionic conductivity ACS Energy Lett. 4 265-70 doi: 10.1021/acsenergylett.8b01997
    [131]
    Zhang Z, Zhang L, Liu Y, Yan X, Xu B, Wang L-M 2020 One-step solution process toward formation of Li6PS5Cl argyrodite solid electrolyte for all-solid-state lithium-ion batteries J. Alloys Compd. 812 152103 doi: 10.1016/j.jallcom.2019.152103
    [132]
    Wissel K, et al 2023 Dissolution and recrystallization behavior of Li3PS4 in different organic solvents with a focus on N-methylformamide ACS Appl. Energy Mater. 6 7790-802 doi: 10.1021/acsaem.2c03278
    [133]
    Ruhl J, Riegger L M, Ghidiu M, Zeier W G 2021 Impact of solvent treatment of the superionic argyrodite Li6PS5Cl on solid-state battery performance Adv. Energy Sustain. Res. 2 2000077 doi: 10.1002/aesr.202000077
    [134]
    Yubuchi S, Uematsu M, Deguchi M, Hayashi A, Tatsumisago M 2018 Lithium-ion-conducting argyrodite-type Li6PS5X (X = Cl, Br, I) solid electrolytes prepared by a liquid-phase technique using ethanol as a solvent ACS Appl. Energy Mater. 1 3622-9 doi: 10.1021/acsaem.8b00280
    [135]
    Azhari L, Bong S, Ma X, Wang Y 2020 Recycling for all solid-state lithium-ion batteries Matter 3 1845-61 doi: 10.1016/j.matt.2020.10.027
    [136]
    Zhu Y, He X, Mo Y 2015 Origin of outstanding stability in the lithium solid electrolyte materials: insights from thermodynamic analyses based on first-principles calculations ACS Appl. Mater. Interfaces 7 23685-93 doi: 10.1021/acsami.5b07517
    [137]
    Morchhale A, Tang Z, Yu C, Farahati R, Kim J-H 2023 Coating materials and processes for cathodes in sulfide-based all solid-state batteries Curr. Opin. Electrochem. 39 101251 doi: 10.1016/j.coelec.2023.101251
    [138]
    Wissel K, Haben A, Kster K, Starke U, Kautenburger R, Ensinger W, Clemens O 2023 Recycling of -Li3PS4-based all-solid-state Li-ion batteries: Interactions of electrode materials and electrolyte in a dissolution-based separation process 10.48550/arxiv.2311.07190
    [139]
    Heubner C, Maletti S, Auer H, Httl J, Voigt K, Lohrberg O, Nikolowski K, Partsch M, Michaelis A 2021 From lithium-metal toward anode-free solid-state batteries: current developments, issues, and challenges Adv. Funct. Mater. 31 2106608 doi: 10.1002/adfm.202106608
    [140]
    Hood Z D, Kates C, Kirkham M, Adhikari S, Liang C, Holzwarth N A W 2016 Structural and electrolyte properties of Li4P2S6 Solid State Ionics 284 61-70 doi: 10.1016/j.ssi.2015.10.015
    [141]
    Wolf G-U, Meisel M 1982 Beitrge zur Chemie von Phosphorverbindungen mit Adamantanstruktur. ber Darstellung und Eigenschaften von Nonathio-cyclotriphosphat Z. Anorg. Allg. Chem. 494 49-54 doi: 10.1002/zaac.19824940106
    [142]
    Sitzmann H, Redaktion R, Schmidt A 2008 Phosphane RÖMPP. Thieme Gruppe(available at: https://roempp.thieme.de/lexicon/RD-16-01853)(Accessed 16 October 2023)
    [143]
    Sitzmann H 2006 Chloride RÖMPP. Thieme Gruppe(available at: https://roempp.thieme.de/lexicon/RD-03-01457)(Accessed 16 October 2023)
    [144]
    Seifert H J 2006 Ternary chlorides of the trivalent late lanthanides J. Therm. Anal. Calorim. 83 479-505 doi: 10.1007/s10973-005-7132-7
    [145]
    Kear G, Barker B D, Walsh F C 2004 Electrochemical corrosion of unalloyed copper in chloride media--a critical review Corros. Sci. 46 109-35 doi: 10.1016/S0010-938X(02)00257-3
    [146]
    Jacob M, Wissel K, Clemens O, et al in preparation
    [147]
    Humani N 2021 Recycling of Li3OCl-based solid-state batteries Bachelor Thesis Institut fr Materialwissenschaft. Chemische MaterialsyntheseUniversity of Stuttgart
    [148]
    Ensing B, Tiwari A, Tros M, Hunger J, Domingos S R, Perez C, Smits G, Bonn M, Bonn D, Woutersen S 2019 On the origin of the extremely different solubilities of polyethers in water Nat. Commun. 10 2893 doi: 10.1038/s41467-019-10783-z
    [149]
    zdemir C, Gner A 2007 Solubility profiles of poly(ethylene glycol)/solvent systems, I: qualitative comparison of solubility parameter approaches Eur. Polym. J. 43 3068-93 doi: 10.1016/j.eurpolymj.2007.02.022
    [150]
    Xin N, Sun Y, He M, Radke C J, Prausnitz J M 2018 Solubilities of six lithium salts in five non-aqueous solvents and in a few of their binary mixtures Fluid Phase Equilib. 461 1-7 doi: 10.1016/j.fluid.2017.12.034
    [151]
    Roth S H 2004 Signal Transduction and the Gasotransmitters: NO, CO, and H2S in Biology and MedicineWang R 2004 Humana Press 293-313 doi: 10.1007/978-1-59259-806-9
    [152]
    Jovell D, Pou J O, Llovell F, Gonzalez-Olmos R 2022 Life cycle assessment of the separation and recycling of fluorinated gases using ionic liquids in a circular economy framework ACS Sustain. Chem. Eng. 10 71-80 doi: 10.1021/acssuschemeng.1c04723
    [153]
    Popp D 2022 (available at: www.europarl.europa.eu/news/en/press-room/20221205IPR60614/batteries-deal-on-new-eu-rules-for-design-production-and-waste-treatment)(Accessed 16 October 2023)
    [154]
    Mao J, Ye C, Zhang S, Xie F, Zeng R, Davey K, Guo Z, Qiao S 2022 Toward practical lithium-ion battery recycling: adding value, tackling circularity and recycling-oriented design Energy Environ. Sci. 15 2732-52 doi: 10.1039/D2EE00162D
    [155]
    Pozo Arcos B, Balkenende A R, Bakker C A, Sundin E 2018 Product design for a circular economy: functional recovery on focus DS 92: Proc. Design 2018 15th Int. Design Conf. 2727-3810.21278/idc.2018.0214
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