Critical state-induced emergence of superior magnetic performances in an iron-based amorphous soft magnetic composite

Liliang Shao; Rongsheng Bai; Yanxue Wu; Jing Zhou; Xing Tong; Hailong Peng; Tao Liang; Zongzhen Li; Qiaoshi Zeng; Bo Zhang; Haibo Ke; Weihua Wang

doi:10.1088/2752-5724/ad2ae8

Volume 3 Issue 2

June 2024

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Article Contents

Liliang Shao, Rongsheng Bai, Yanxue Wu, Jing Zhou, Xing Tong, Hailong Peng, Tao Liang, Zongzhen Li, Qiaoshi Zeng, Bo Zhang, Haibo Ke, Weihua Wang. Critical state-induced emergence of superior magnetic performances in an iron-based amorphous soft magnetic composite[J]. Materials Futures, 2024, 3(2): 025301. doi: 10.1088/2752-5724/ad2ae8

Citation:

Liliang Shao, Rongsheng Bai, Yanxue Wu, Jing Zhou, Xing Tong, Hailong Peng, Tao Liang, Zongzhen Li, Qiaoshi Zeng, Bo Zhang, Haibo Ke, Weihua Wang. Critical state-induced emergence of superior magnetic performances in an iron-based amorphous soft magnetic composite[J]. Materials Futures, 2024, 3(2): 025301. doi: 10.1088/2752-5724/ad2ae8

Citation:

Liliang Shao, Rongsheng Bai, Yanxue Wu, Jing Zhou, Xing Tong, Hailong Peng, Tao Liang, Zongzhen Li, Qiaoshi Zeng, Bo Zhang, Haibo Ke, Weihua Wang. Critical state-induced emergence of superior magnetic performances in an iron-based amorphous soft magnetic composite[J]. Materials Futures, 2024, 3(2): 025301. doi: 10.1088/2752-5724/ad2ae8

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Critical state-induced emergence of superior magnetic performances in an iron-based amorphous soft magnetic composite

Materials Futures, Volume 3, Number 2

Received Date: 2023-12-14
Accepted Date: 2024-02-20
Publish Date: 2024-03-05

Article information

doi: 10.1088/2752-5724/ad2ae8

1 Songshan Lake Materials Laboratory, Dongguan 523808, People’s Republic of China
2 Institute of Physics, Chinese Academy of Sciences, Beijing 100190, People’s Republic of China
3 School of Energy, Power and Mechanical Engineering, North China Electric Power University, Beijing 100096, People’s Republic of China
4 School of Materials Science and Engineering, Central South University, Changsha 410083, People’s Republic of China
5 Center for High Pressure Science and Technology Advanced Research, Shanghai 201203, People’s Republic of China
6 Jiangsu JITRI Advanced Energy Materials Research Institute Co., Ltd, Changzhou 213000, People’s Republic of China
Co-first authors: Liliang Shao, Rongsheng Bai

Funds:

This work was financially supported by Guangdong Major Project of Basic and Applied Basic Research, China (Grant No. 2019B030302010), the National Natural Science Foundation of China (Grant Nos. 52301212, 52071222, 52101191, 52001219), the National Key Research and Development Program of China (Grant No. 2021YFA0716302), and Guangdong Basic and Applied Basic Research, China (Grant Nos. 2022A1515010347, 2020B1515130007).

Abstract

Abstract

Soft magnetic composites (SMCs) play a pivotal role in the development of high-frequency, miniaturization and complex forming of modern electronics. However, they usually suffer from a trade-off between high magnetization and good magnetic softness (high permeability and low core loss). In this work, utilizing the order modulation strategy, a critical state in a FeSiBCCr amorphous soft magnetic composite (ASMC), consisting of massive crystal-like orders (CLOs, ∼1 nm in size) with the feature of α-Fe, is designed. This critical-state structure endows the amorphous powder with the enhanced ferromagnetic exchange interactions and the optimized magnetic domains with uniform orientation and fewer micro-vortex dots. Superior comprehensive soft magnetic properties at high frequency emerge in the ASMC, such as a high saturation magnetization (M_s) of 170 emu g⁻¹ and effective permeability (μ_e) of 65 combined with a core loss (P_cv) as low as 70 mW cm⁻³ (0.01 T, 1 MHz). This study provides a new strategy for the development of high-frequency ASMCs, possessing suitable comprehensive soft magnetic performance to match the requirements of the modern magnetic devices used in the third-generation semiconductors and new energy fields.
- amorphous soft magnetic composites,
- critical state,
- soft magnetic property,
- rotating magnetic field annealing,
- magnetic domain

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References(55)

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